{"paper":{"title":"Determination of Hund's coupling in 5d Oxides using Resonant Inelastic X-ray Scattering","license":"http://arxiv.org/licenses/nonexclusive-distrib/1.0/","headline":"","cross_cats":[],"primary_cat":"cond-mat.str-el","authors_text":"A. M. Cook, Arun Paramekanti, B.-C. Jeon, Bo Yuan, C. M. Thompson, D. Casa, G. Cao, J. Greedan, J. P. Clancy, M. H. Upton, T. Gog, T.-W. Noh, Young-June Kim","submitted_at":"2017-01-23T19:00:30Z","abstract_excerpt":"We report resonant inelastic X-ray scattering (RIXS) measurements on ordered double perovskite samples containing Re$^{5+}$ and Ir$^{5+}$ with $5d^2$ and $5d^4$ electronic configurations respectively. In particular, the observed RIXS spectra of Ba$_2$YReO$_6$ and Sr$_2$MIrO$_6$ (M=Y, Gd) show sharp intra-t$_{2g}$ transitions, which can be quantitatively understood using a minimal `atomic' Hamiltonian incorporating spin-orbit coupling ($\\lambda$) and Hund's coupling ($J_H$). Our analysis yields $\\lambda=0.38(2)$eV with $J_H=0.26(2)$eV for Re$^{5+}$, and $\\lambda=0.42(2)$eV with $J_H=0.25(4)$eV "},"claims":{"count":0,"items":[],"snapshot_sha256":"258153158e38e3291e3d48162225fcdb2d5a3ed65a07baac614ab91432fd4f57"},"source":{"id":"1701.06584","kind":"arxiv","version":3},"verdict":{"id":null,"model_set":{},"created_at":null,"strongest_claim":"","one_line_summary":"","pipeline_version":null,"weakest_assumption":"","pith_extraction_headline":""},"references":{"count":0,"sample":[],"resolved_work":0,"snapshot_sha256":"258153158e38e3291e3d48162225fcdb2d5a3ed65a07baac614ab91432fd4f57","internal_anchors":0},"formal_canon":{"evidence_count":0,"snapshot_sha256":"258153158e38e3291e3d48162225fcdb2d5a3ed65a07baac614ab91432fd4f57"},"author_claims":{"count":0,"strong_count":0,"snapshot_sha256":"258153158e38e3291e3d48162225fcdb2d5a3ed65a07baac614ab91432fd4f57"},"builder_version":"pith-number-builder-2026-05-17-v1"}