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arxiv: 1709.04930 · v4 · pith:M4FJWGXMnew · submitted 2017-09-14 · ❄️ cond-mat.soft · cond-mat.dis-nn· cond-mat.mtrl-sci

Low-temperature anomalies of a vapor deposited glass

classification ❄️ cond-mat.soft cond-mat.dis-nncond-mat.mtrl-sci
keywords anomaliesglassvaporcoolingdepositionfilmsliquidprepared
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We investigate the low temperature properties of two-dimensional Lennard-Jones glass films, prepared in silico both by liquid cooling and by physical vapor deposition. We identify deep in the solid phase a crossover temperature $T^*$, at which slow dynamics and enhanced heterogeneity emerge. Around $T^*$, localized defects become visible, leading to vibrational anomalies as compared to standard solids. We find that on average, $T^*$ decreases in samples with lower inherent structure energy, suggesting that such anomalies will be suppressed in ultra-stable glass films, prepared both by very slow liquid cooling and vapor deposition.

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