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arxiv: 1008.0942 · v3 · pith:QECFXO5Wnew · submitted 2010-08-05 · ❄️ cond-mat.str-el · cond-mat.mtrl-sci

Preformed excitonic liquid route to a charge density wave in 2H-TaSe₂

classification ❄️ cond-mat.str-el cond-mat.mtrl-sci
keywords densitychargeh-tasepreformedwavearisingexcitonicliquid
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Recent experiments on 2H-TaSe$_2$ contradict the long-held view of the charge density wave arising from a nested band structure. An intrinsically strong coupling view, involving a charge density wave state arising as a Bose condensation of preformed excitons emerges as an attractive, albeit scantily investigated alternative. Using local density approximation plus multiorbital dynamic mean-field theory, we show that this scenario agrees with a variety of normal state data for 2H-TaSe$_{2}$. Based thereupon, the ordered states in a subset of dichalcogenides should be viewed as instabilities of a correlated, preformed excitonic liquid.

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