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arxiv: 1907.01234 · v1 · pith:WOEHTB7Mnew · submitted 2019-07-02 · ⚛️ physics.atom-ph · quant-ph

Electric Rydberg-atom interferometery

Pith reviewed 2026-05-25 10:42 UTC · model grok-4.3

classification ⚛️ physics.atom-ph quant-ph
keywords Rydberg atomsmatter-wave interferometryinhomogeneous electric fieldsHahn echo sequencehelium atomscircular Rydberg statesStern-Gerlach interferometermicrowave pulses
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0 comments X

The pith

A Hahn-echo sequence of microwave pulses and inhomogeneous electric field gradients creates two interfering Rydberg atom matter waves in helium.

A machine-rendered reading of the paper's core claim, the machinery that carries it, and where it could break.

The paper shows how to build an electric version of the longitudinal Stern-Gerlach interferometer using atoms excited to high-n circular Rydberg states. Helium atoms start in a microwave-driven superposition of the n=55 and n=56 states, then experience two identical pulses of an inhomogeneous electric field separated by a microwave inversion pulse. The sequence leaves the atoms in two spatially separated momentum components whose recombination produces clear oscillations in the final state populations when the gradient strength is scanned. A reader would care because the method uses only electric fields and microwaves to split and recombine atomic de Broglie waves, offering a route to matter-wave interferometry that avoids magnetic fields.

Core claim

The experiments realized an electric analogue of the longitudinal Stern-Gerlach matter-wave interferometer. Rydberg helium atoms prepared in coherent superpositions of the n=55 and n=56 circular states were subjected to a Hahn-echo microwave pulse sequence interspersed with a pair of equivalent inhomogeneous electric field pulses. This produced two spatially separated matter waves whose interference appeared as oscillations in the final Rydberg state populations when the amplitude of the pulsed electric field gradients was varied.

What carries the argument

The Hahn-echo microwave pulse sequence (pi/2 - pi - pi/2) with two identical inhomogeneous electric field pulses inserted between the microwave pulses, which first creates a momentum superposition and later equalizes the momenta of the two internal-state components.

If this is right

  • Two spatially separated matter waves are generated from the initial Rydberg superposition.
  • Interference between those waves appears directly as oscillations in the final Rydberg populations.
  • The oscillation period is controlled by the strength of the applied electric field gradient.
  • The same electric-field pulses can be used both to split and to recombine the motional states.
  • The technique works for atoms prepared in high-n circular Rydberg states of helium.

Where Pith is reading between the lines

These are editorial extensions of the paper, not claims the author makes directly.

  • The approach could be adapted to sense small electric field gradients by monitoring the phase of the observed population oscillations.
  • Because the splitting relies only on electric fields, the method may be useful in regions where magnetic fields must be avoided.
  • The same pulse sequence might be applied to other atomic species or lower principal quantum numbers to test the limits of coherence.
  • Extending the gradient pulses to three dimensions could enable full three-dimensional electric atom interferometry.

Load-bearing premise

The inhomogeneous electric field pulses create a clean momentum superposition in the Rydberg atoms without introducing significant decoherence or unwanted state couplings.

What would settle it

If scans of the electric field gradient amplitude show no oscillations in the measured final-state populations, the claim that the sequence produces observable interference between the separated matter waves would be ruled out.

Figures

Figures reproduced from arXiv: 1907.01234 by J. E. Palmer, S. D. Hogan.

Figure 1
Figure 1. Figure 1: FIG. 1. Schematic diagram of the experimental apparatus [PITH_FULL_IMAGE:figures/full_fig_p002_1.png] view at source ↗
Figure 2
Figure 2. Figure 2: FIG. 2. (a) Sequence of electric field and microwave pulses. [PITH_FULL_IMAGE:figures/full_fig_p002_2.png] view at source ↗
Figure 3
Figure 3. Figure 3: FIG. 3. (a) Measured, and (b) calculated Rydberg-atom in [PITH_FULL_IMAGE:figures/full_fig_p003_3.png] view at source ↗
Figure 4
Figure 4. Figure 4: FIG. 4. Effects of modifications to the microwave and elec [PITH_FULL_IMAGE:figures/full_fig_p004_4.png] view at source ↗
read the original abstract

An electric analogue of the longitudinal Stern-Gerlach matter-wave interferometer has been realized for atoms in Rydberg states with high principal quantum number, $n$. The experiments were performed with He atoms prepared in coherent superpositions of the $n=55$ and $n=56$ circular Rydberg states in zero electric field by a $\pi/2$ pulse of resonant microwave radiation. These atoms were subjected to a pulsed inhomogeneous electric field to generate a superposition of momentum states before a $\pi$ pulse was applied to invert the internal states. The same pulsed inhomogeneous electric field was then reapplied for a second time to transform the motional states to have equal momenta before a further $\pi/2$ pulse was employed to interrogate the final Rydberg state populations. This Hahn-echo microwave pulse sequence, interspersed with a pair of equivalent inhomogeneous electric field pulses, yielded two spatially separated matter waves. Interferences between these matter waves were observed as oscillations in the final Rydberg state populations as the amplitude of the pulsed electric field gradients was adjusted.

Editorial analysis

A structured set of objections, weighed in public.

Desk editor's note, referee report, simulated authors' rebuttal, and a circularity audit. Tearing a paper down is the easy half of reading it; the pith above is the substance, this is the friction.

Referee Report

2 major / 0 minor

Summary. The paper reports the experimental realization of an electric analogue of the longitudinal Stern-Gerlach matter-wave interferometer for helium atoms in high-n circular Rydberg states (n=55 and n=56). A Hahn-echo sequence of resonant microwave π/2, π, and π/2 pulses is interspersed with two equivalent pulsed inhomogeneous electric fields; the authors claim this produces two spatially separated matter waves whose interference manifests as oscillations in the final Rydberg-state populations when the amplitude of the electric-field gradients is varied.

Significance. If the observations hold, the work demonstrates a new electric-field-based approach to Rydberg-atom interferometry that exploits the large electric dipole moments of circular states. This could enable precision electrometry or coherence studies without magnetic fields. The use of a Hahn-echo sequence to refocus internal states while manipulating motion is a conceptually clean idea, but the manuscript supplies no quantitative data, figures, error bars, or statistical analysis to support the interference claim.

major comments (2)
  1. [Abstract / experimental procedure] Abstract and experimental description: the central claim that 'interferences between these matter waves were observed as oscillations' is presented without any quantitative data, error bars, figures, or statistical analysis of the population oscillations versus gradient amplitude. This absence directly undermines evaluation of the result.
  2. [Experimental procedure] Experimental procedure description: the implicit assumption that the inhomogeneous electric-field pulses produce a clean momentum-state superposition without significant decoherence or unwanted couplings is not supported by any controls, lifetime measurements, or auxiliary data, yet this assumption is load-bearing for the interference observation.

Simulated Author's Rebuttal

2 responses · 0 unresolved

We thank the referee for their careful reading of the manuscript and for highlighting these important points regarding the presentation of our experimental results. We address each major comment below.

read point-by-point responses
  1. Referee: [Abstract / experimental procedure] Abstract and experimental description: the central claim that 'interferences between these matter waves were observed as oscillations' is presented without any quantitative data, error bars, figures, or statistical analysis of the population oscillations versus gradient amplitude. This absence directly undermines evaluation of the result.

    Authors: We agree that the manuscript as submitted does not include quantitative data, figures, error bars or statistical analysis to support the claimed oscillations in final-state populations. This is a valid criticism that weakens the ability to evaluate the central claim. In the revised manuscript we will add the relevant experimental figures showing population versus gradient amplitude, together with error bars and a description of the statistical analysis. revision: yes

  2. Referee: [Experimental procedure] Experimental procedure description: the implicit assumption that the inhomogeneous electric-field pulses produce a clean momentum-state superposition without significant decoherence or unwanted couplings is not supported by any controls, lifetime measurements, or auxiliary data, yet this assumption is load-bearing for the interference observation.

    Authors: The referee correctly notes that the manuscript provides no auxiliary data or controls to substantiate the assumption of clean momentum-state superposition. We will revise the experimental-procedure section to include available lifetime measurements and any control data demonstrating that decoherence and unwanted couplings remain negligible under the applied field pulses. revision: yes

Circularity Check

0 steps flagged

No significant circularity

full rationale

The paper reports an experimental realization of a Rydberg-atom interferometer via a Hahn-echo microwave sequence with pulsed inhomogeneous electric fields. The abstract and described content contain no equations, derivations, fitted parameters, or self-citations that could form a load-bearing chain. The central claim rests on direct observation of population oscillations, with no reduction of predictions to inputs by construction. This matches the reader's assessment of circularity score 0.0 and indicates a self-contained experimental report.

Axiom & Free-Parameter Ledger

0 free parameters · 2 axioms · 0 invented entities

The work rests on standard domain assumptions about Rydberg-state preparation and electric-field interactions with no new entities or fitted parameters introduced in the abstract.

axioms (2)
  • domain assumption Coherent superpositions of circular Rydberg states can be created and inverted with resonant microwave pulses
    Explicitly stated as performed by the π/2 and π pulses.
  • domain assumption Inhomogeneous electric field pulses impart state-dependent momentum shifts sufficient to create spatially separated matter waves
    Required for the interferometer to function as described.

pith-pipeline@v0.9.0 · 5704 in / 1258 out tokens · 65210 ms · 2026-05-25T10:42:19.709300+00:00 · methodology

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Works this paper leans on

53 extracted references · 53 canonical work pages

  1. [1]

    Gerlach and O

    W. Gerlach and O. Stern, Der experimentelle Nachweis des magnetischen Moments des Silberatoms, Z. Phys. 8, 110 (1922)

  2. [2]

    Gerlach and O

    W. Gerlach and O. Stern, Der experimentelle Nachweis der Richtungsquantelung im Magnetfeld, Z. Phys. 9, 349 (1922)

  3. [3]

    I. I. Rabi, J. R. Zacharias, S. Millman, and P. Kusch, A New Method of Measuring Nuclear Magnetic Moment, Phys. Rev. 53, 318 (1938)

  4. [4]

    J. W. Emsley and J. Feeney, Forty years of Progress in Nuclear Magnetic Resonance Spectroscopy, Prog. Nucl. Magn. Reson. Spectrosc. 50, 179 (2007)

  5. [5]

    H. G. Bennewitz, W. Paul and Ch. Schlier, Fokussierung polarer Molek¨ ule, Z. Phys.141, 6 (1955)

  6. [6]

    J. P. Gordon, H. J. Zeiger, and C. H. Townes, The Maser – New Type of Microwave Amplifier, Frequency Stan- dard, and Spectrometer, Phys. Rev. 99, 1264 (1955)

  7. [7]

    Migdall, John V

    Alan L. Migdall, John V. Prodan, William D. Phillips, Thomas H. Bergeman, and Harold J. Metcalf, First Ob- servation of Magnetically Trapped Neutral Atoms, Phys. Rev. Lett. 54, 2596 (1985)

  8. [8]

    E. A. Cornell and C. E. Wieman, Nobel Lecture: Bose- Einstein condensation in a dilute gas, the first 70 years and some recent experiments, Rev. Mod. Phys. 74, 875 (2002)

  9. [9]

    Ketterle, Nobel lecture: When atoms behave as waves: Bose-Einstein condensation and the atom laser, Rev

    W. Ketterle, Nobel lecture: When atoms behave as waves: Bose-Einstein condensation and the atom laser, Rev. Mod. Phys. 74, 1131 (2002)

  10. [10]

    H. L. Bethlem, G. Berden, and G. Meijer, Decelerating Neutral Dipolar Molecules, Phys. Rev. Lett. 83, 1558 (1999)

  11. [11]

    Vanhaecke, U

    N. Vanhaecke, U. Meier, M. Andrist, B. H. Meier, and F.Merkt, Multistage Zeeman deceleration of hydrogen atoms, Phys. Rev. A 75, 031402(R) (2007)

  12. [12]

    Narevicius, C

    E. Narevicius, C. G. Parthey, A. Libson, J. Narevicius, I. Chavez, U. Even, and M. G. Raizen, An atomic coilgun: using pulsed magnetic fields to slow a supersonic beam, New J. Phys. 9, 358 (2007 )

  13. [13]

    J. J. Gilijamse, S. Hoekstra, S. Y. T. van de Meerakker, G. C. Groenenboom, and G. Meijer, Near-Threshold In- elastic Collisions Using Molecular Beams with a Tunable Velocity, Science 313, 1617 (2006)

  14. [14]

    von Zastrow, J

    A. von Zastrow, J. Onvlee, S. N. Vogels, G. C. Groenen- boom, A. van der Avoird, and S. Y. T. van de Meerakker, State-resolved diffraction oscillations imaged for inelas- tic collisions of NO radicals with He, Ne and Ar, Nature Chemistry 6, 216 (2014)

  15. [15]

    Allmendinger, J

    P. Allmendinger, J. Deiglmayr, K. H¨ oveler, O. Schullian, and F. Merkt, Observation of enhanced rate coefficients in the H + 2 + H2 → H+ 3 + H reaction at low collision ener- gies, J. Chem. Phys. 145, 244316 (2016)

  16. [16]

    van Veldhoven, J

    J. van Veldhoven, J. K¨ upper, H. L. Bethlem, B. Sartakov, A. J.A. van Roij, and G. Meijer, Decelerated molecular beams for high-resolution spectroscopy – The hyperfine structure of 15ND3, Eur. Phys. J. D 31, 337 (2004)

  17. [17]

    Jansen, L

    P. Jansen, L. Semeria, L. Esteban Hofer, S. Scheideg- ger, J. A. Agner, H. Schmutz, and F. Merkt, Precision Spectroscopy in Cold Molecules: The Lowest Rotational Interval of He + 2 and Metastable He 2, Phys. Rev. Lett. 115, 133202 (2015)

  18. [18]

    Jansen, L

    P. Jansen, L. Semeria, and F. Merkt, Determination of the Spin-Rotation Fine Structure of He + 2 , Phys. Rev. Lett. 120, 043001 (2018)

  19. [19]

    H. L. Bethlem, F. M. H. Crompvoets, R. T. Jongma, S. Y. T. van de Meerakker, and G. Meijer, Deceleration and trapping of ammonia using time-varying electric fields, Phys. Rev. A 65, 053416 (2002)

  20. [20]

    S. D. Hogan and F. Merkt, Demonstration of Three- Dimensional Electrostatic Trapping of State-Selected Ry- dberg Atoms, Phys. Rev. Lett. 100, 043001 (2008)

  21. [21]

    J. J. Gilijamse, S. Hoekstra, S. A. Meek, M. Mets¨ al¨ a, S. Y. T. van de Meerakker, G. Meijer, and G. C. Groenen- boom, The radiative lifetime of metastable CO (a 3Π), J. Chem. Phys. 127, 221102 (2007)

  22. [22]

    S. Y. T. van de Meerakker, N. Vanhaecke, M. P. J. van der Loo, G. C. Groenenboom, and G. Meijer, Direct Mea- surement of the Radiative Lifetime of Vibrationally Ex- cited OH Radicals, Phys. Rev. Lett. 95, 013003 (2005)

  23. [23]

    Seiler, S

    Ch. Seiler, S. D. Hogan, H. Schmutz, J. A. Agner, and F. Merkt, Collisional and Radiative Processes in Adia- batic Deceleration, Deflection, and Off-Axis Trapping of a Rydberg Atom Beam, Phys. Rev. Lett. 106, 073003 (2011)

  24. [24]

    Seiler, J

    Ch. Seiler, J. A. Agner, P. Pillet, and F Merkt, Radiative and collisional processes in translationally cold samples of hydrogen Rydberg atoms studied in an electrostatic trap, J. Phys. B 49, 094006 (2016)

  25. [25]

    Bohm, Quantum Theory , Prentice-Hall, New York (1951)

    D. Bohm, Quantum Theory , Prentice-Hall, New York (1951)

  26. [26]

    E. P. Wigner, The Problem of Measurement, Am. J. Phys. 31, 6 (1963)

  27. [27]

    Schwinger, M

    J. Schwinger, M. O. Scully, and B.-G. Englert, Is spin co- herence like Humpty-Dumpty?, Z Phys. D10, 135 (1988)

  28. [28]

    Y. L. Sokolov, Influence of Lamb shift on the interference of excited states of hydrogen atoms, JETP Lett. 11, 359 (1970) 6

  29. [29]

    Y. L. Sokolov, Interference of the 2p 1/2 state of the hy- drogen atom, Sov. Phys. JETP 36, 243 (1973)

  30. [30]

    Miniatura, F

    Ch. Miniatura, F. Perales, G. Vassilev, J. Reinhardt, J. Robert and J. Baudon, A longitudinal Stern-Gerlach in- terferometer : the “beaded” atom, J. Phys. II France 1, 425 (1991)

  31. [31]

    Miniatura, J

    Ch. Miniatura, J. Robert, O. Gorceix, V. Lorent, S. Le Boiteux, J. Reinhardt, and J. Baudon, Atomic interfer- ences and the topological phase, Phys. Rev. Lett. 69, 261 (1992)

  32. [32]

    S Nic Chormaic, V Wiedemann, C Miniatura, J Robert, S Le Boiteux, V Lorent, O Gorceix, S Feron, J Reinhardt and J Baudon, Longitudinal Stern-Gerlach atomic inter- ferometry using velocity selected atomic beams, J. Phys. B 26, 1271 (1993)

  33. [33]

    Machluf, Y

    S. Machluf, Y. Japha, and R. Folman, Coherent Stern- Gerlach momentum splitting on an atom chip, Nat. Com- mun. 4, 2424 (2013)

  34. [34]

    A. D. Cronin, J. Schmiedmayer, and D. E. Pritchard, Op- tics and interferometry with atoms and molecules, Rev. Mod. Phys. 81, 1051 (2009)

  35. [35]

    Hornberger, S

    K. Hornberger, S. Gerlich, P. Haslinger, S. Nimmrichter, and M. Arndt, M., Colloquium: Quantum interference of clusters and molecules, Rev. Mod. Phys. 84, 157 (2012)

  36. [36]

    Townsend, A

    D. Townsend, A. L. Goodgame, S. R. Procter, S. R. Mackenzie, and T. P. Softley, Deflection of krypton Ry- dberg atoms in the field of an electric dipole, J. Phys. B 34, 439 (2001)

  37. [37]

    S. D. Hogan, Rydberg-Stark deceleration of atoms and molecules, EPJ Techniques and Instrumentation 3, 1 (2016)

  38. [38]

    D. B. Cassidy, Experimental progress in positronium laser physics, Eur. Phys. J. D 72, 53 (2018)

  39. [39]

    N. F. Ramsey, Experiments with separated oscillatory fields and hydrogen masers, Rev. Mod. Phys. 62, 541 (1990)

  40. [40]

    J. M. Raimond, M. Brune, and S. Haroche, Manipulat- ing quantum entanglement with atoms and photons in a cavity, Rev. Mod. Phys. 73, 565 (2001)

  41. [41]

    Kellerbauer, M

    A. Kellerbauer, M. Amoretti, A. S. Belov, G. Bonomi, I. Boscolo, R. S. Brusa, M. B¨ uchner, V. M. Byakov, L. Cabaret, C. Canali, C. Carraro, F. Castelli, S. Cialdi, M. de Combarieu, D. Comparat, G. Consolati, N. Djourelov, M. Doser, G. Drobychev, A. Dupasquier, G. Ferrari, P. Forget, L. Formaro, A. Gervasini, M. G. Giammarchi, S. N. Gninenko, G. Gribakin,...

  42. [42]

    Amole, M

    C. Amole, M. D. Ashkezari, M. Baquero-Ruiz, W. Bertsche, E. Butler, A. Capra, C. L. Cesar, M. Charl- ton, S. Eriksson, J. Fajans, T. Friesen, M. C. Fujiwara, D. R. Gill, A. Gutierrez, J. S. Hangst, W. N. Hardy, M. E. Hayden, C. A. Isaac, S. Jonsell, L. Kurchaninov, A. Little, N. Madsen, J. T. K. McKenna, S. Menary, S. C. Napoli, P. Nolan, A. Olin, P. Pusa...

  43. [43]

    A. P. Mills, Jr. and M. Leventhal, Can we measure the gravitational free fall of cold Rydberg state positronium?, Nucl. Instrum. Methods Phys. Res., Sect. B 192, 102 (2002)

  44. [44]

    D. B. Cassidy and S. D. Hogan, Atom control and gravity measurements using Rydberg positronium, Int. J. Mod. Phys. Conf. Ser. 30, 1460259 (2014)

  45. [45]

    Bassi, K

    A. Bassi, K. Lochan, S. Satin, T. P. Singh, and H. Ul- bricht, Models of wave-function collapse, underlying the- ories, and experimental tests, Rev. Mod. Phys. 85, 471 (2013)

  46. [46]

    Delande and J

    D. Delande and J. C. Gay, A New Method for Producing Circular Rydberg States, Euro. Phys. Lett. 5, 303 (1988)

  47. [47]

    Zhelyazkova and S

    V. Zhelyazkova and S. D. Hogan, Preparation of circular Rydberg states in helium using the crossed-fields method, Phys. Rev. A 94, 023415 (2016)

  48. [48]

    S. D. Hogan, Y. Houston, and B. Wei, Laser photoexcita- tion of Rydberg states in helium with n> 400, J. Phys. B 51, 145002 (2018)

  49. [49]

    R. J. Elliott, G. Droungas, and J.-P. Connerade, Active cancellation of the motional Stark effect in the diamag- netic spectrum of Ba, J. Phys. B 28, L537 (1995)

  50. [50]

    J. E. Palmer and S. D. Hogan, Matter-wave interferom- etry with atoms in high Rydberg states, Mol. Phys., In Press (2019)

  51. [51]

    Pauli, ¨Uber das Wasserstoffspektrum vom Stand- punkt der neuen Quantenmechanik, Z

    W. Pauli, ¨Uber das Wasserstoffspektrum vom Stand- punkt der neuen Quantenmechanik, Z. Phys. 36, 336 (1926)

  52. [52]

    Ch. J. Bord´ e, Atomic interferometry with internal state labeling, Phys. Lett. A, 140, 10 (1989)

  53. [53]

    Deller, A

    A. Deller, A. M. Alonso, B. S. Cooper, S. D. Hogan, and D. B. Cassidy, Measurement of Rydberg positronium fluorescence lifetimes, Phys. Rev. A 93, 062513 (2016)