{"record_type":"pith_number_record","schema_url":"https://pith.science/schemas/pith-number/v1.json","pith_number":"pith:2017:3BFJ4NWGM6QAJ6HTVMJ3422AAL","short_pith_number":"pith:3BFJ4NWG","schema_version":"1.0","canonical_sha256":"d84a9e36c667a004f8f3ab13be6b4002d4672d637c1307f7a87fbdcaeeaea4aa","source":{"kind":"arxiv","id":"1711.11242","version":1},"attestation_state":"computed","paper":{"title":"Theory for Nonlinear Spectroscopy of Vibrational Polaritons","license":"http://arxiv.org/licenses/nonexclusive-distrib/1.0/","headline":"","cross_cats":["physics.chem-ph"],"primary_cat":"quant-ph","authors_text":"Adam D. Dunkelberger, Blake S. Simpkins, Bo Xiang, Jeffrey C. Owrutsky, Joel Yuen-Zhou, Raphael F. Ribeiro, Wei Xiong","submitted_at":"2017-11-30T05:44:59Z","abstract_excerpt":"Molecular polaritons have gained considerable attention due to their potential to control nanoscale molecular processes by harnessing electromagnetic coherence. Although recent experiments with liquid-phase vibrational polaritons have shown great promise for exploiting these effects, significant challenges remain in interpreting their spectroscopic signatures. In this letter, we develop a quantum-mechanical theory of pump-probe spectroscopy for this class of polaritons based on the quantum Langevin equations and the input-output theory. Comparison with recent experimental data shows good agree"},"verification_status":{"content_addressed":true,"pith_receipt":true,"author_attested":false,"weak_author_claims":0,"strong_author_claims":0,"externally_anchored":false,"storage_verified":false,"citation_signatures":0,"replication_records":0,"graph_snapshot":true,"references_resolved":false,"formal_links_present":false},"canonical_record":{"source":{"id":"1711.11242","kind":"arxiv","version":1},"metadata":{"license":"http://arxiv.org/licenses/nonexclusive-distrib/1.0/","primary_cat":"quant-ph","submitted_at":"2017-11-30T05:44:59Z","cross_cats_sorted":["physics.chem-ph"],"title_canon_sha256":"12aa4a2d0f3c73d2beacdfd0088149e6c1d7d3b35bfb8e136ef0897e638196b1","abstract_canon_sha256":"ddc1669e27d43c18ae80cbdac12f7070c55be4e1935544c24620b96e4a73f2c1"},"schema_version":"1.0"},"receipt":{"kind":"pith_receipt","key_id":"pith-v1-2026-05","algorithm":"ed25519","signed_at":"2026-05-18T00:29:12.088000Z","signature_b64":"JfFnX2RCJsRp1HjCgvgBjQKTvZe++UdgDvFV8Jy4qFQ0v9IMmGMmrTR/C8yVEIO/4fBZfdCxPM+wulS9M1j7DA==","signed_message":"canonical_sha256_bytes","builder_version":"pith-number-builder-2026-05-17-v1","receipt_version":"0.3","canonical_sha256":"d84a9e36c667a004f8f3ab13be6b4002d4672d637c1307f7a87fbdcaeeaea4aa","last_reissued_at":"2026-05-18T00:29:12.087467Z","signature_status":"signed_v1","first_computed_at":"2026-05-18T00:29:12.087467Z","public_key_fingerprint":"8d4b5ee74e4693bcd1df2446408b0d54"},"graph_snapshot":{"paper":{"title":"Theory for Nonlinear Spectroscopy of Vibrational Polaritons","license":"http://arxiv.org/licenses/nonexclusive-distrib/1.0/","headline":"","cross_cats":["physics.chem-ph"],"primary_cat":"quant-ph","authors_text":"Adam D. Dunkelberger, Blake S. Simpkins, Bo Xiang, Jeffrey C. Owrutsky, Joel Yuen-Zhou, Raphael F. Ribeiro, Wei Xiong","submitted_at":"2017-11-30T05:44:59Z","abstract_excerpt":"Molecular polaritons have gained considerable attention due to their potential to control nanoscale molecular processes by harnessing electromagnetic coherence. Although recent experiments with liquid-phase vibrational polaritons have shown great promise for exploiting these effects, significant challenges remain in interpreting their spectroscopic signatures. In this letter, we develop a quantum-mechanical theory of pump-probe spectroscopy for this class of polaritons based on the quantum Langevin equations and the input-output theory. Comparison with recent experimental data shows good agree"},"claims":{"count":0,"items":[],"snapshot_sha256":"258153158e38e3291e3d48162225fcdb2d5a3ed65a07baac614ab91432fd4f57"},"source":{"id":"1711.11242","kind":"arxiv","version":1},"verdict":{"id":null,"model_set":{},"created_at":null,"strongest_claim":"","one_line_summary":"","pipeline_version":null,"weakest_assumption":"","pith_extraction_headline":""},"references":{"count":0,"sample":[],"resolved_work":0,"snapshot_sha256":"258153158e38e3291e3d48162225fcdb2d5a3ed65a07baac614ab91432fd4f57","internal_anchors":0},"formal_canon":{"evidence_count":0,"snapshot_sha256":"258153158e38e3291e3d48162225fcdb2d5a3ed65a07baac614ab91432fd4f57"},"author_claims":{"count":0,"strong_count":0,"snapshot_sha256":"258153158e38e3291e3d48162225fcdb2d5a3ed65a07baac614ab91432fd4f57"},"builder_version":"pith-number-builder-2026-05-17-v1"},"aliases":[{"alias_kind":"arxiv","alias_value":"1711.11242","created_at":"2026-05-18T00:29:12.087562+00:00"},{"alias_kind":"arxiv_version","alias_value":"1711.11242v1","created_at":"2026-05-18T00:29:12.087562+00:00"},{"alias_kind":"doi","alias_value":"10.48550/arxiv.1711.11242","created_at":"2026-05-18T00:29:12.087562+00:00"},{"alias_kind":"pith_short_12","alias_value":"3BFJ4NWGM6QA","created_at":"2026-05-18T12:30:58.224056+00:00"},{"alias_kind":"pith_short_16","alias_value":"3BFJ4NWGM6QAJ6HT","created_at":"2026-05-18T12:30:58.224056+00:00"},{"alias_kind":"pith_short_8","alias_value":"3BFJ4NWG","created_at":"2026-05-18T12:30:58.224056+00:00"}],"events":[],"event_summary":{},"paper_claims":[],"inbound_citations":{"count":0,"internal_anchor_count":0,"sample":[]},"formal_canon":{"evidence_count":0,"sample":[],"anchors":[]},"links":{"html":"https://pith.science/pith/3BFJ4NWGM6QAJ6HTVMJ3422AAL","json":"https://pith.science/pith/3BFJ4NWGM6QAJ6HTVMJ3422AAL.json","graph_json":"https://pith.science/api/pith-number/3BFJ4NWGM6QAJ6HTVMJ3422AAL/graph.json","events_json":"https://pith.science/api/pith-number/3BFJ4NWGM6QAJ6HTVMJ3422AAL/events.json","paper":"https://pith.science/paper/3BFJ4NWG"},"agent_actions":{"view_html":"https://pith.science/pith/3BFJ4NWGM6QAJ6HTVMJ3422AAL","download_json":"https://pith.science/pith/3BFJ4NWGM6QAJ6HTVMJ3422AAL.json","view_paper":"https://pith.science/paper/3BFJ4NWG","resolve_alias":"https://pith.science/api/pith-number/resolve?arxiv=1711.11242&json=true","fetch_graph":"https://pith.science/api/pith-number/3BFJ4NWGM6QAJ6HTVMJ3422AAL/graph.json","fetch_events":"https://pith.science/api/pith-number/3BFJ4NWGM6QAJ6HTVMJ3422AAL/events.json","actions":{"anchor_timestamp":"https://pith.science/pith/3BFJ4NWGM6QAJ6HTVMJ3422AAL/action/timestamp_anchor","attest_storage":"https://pith.science/pith/3BFJ4NWGM6QAJ6HTVMJ3422AAL/action/storage_attestation","attest_author":"https://pith.science/pith/3BFJ4NWGM6QAJ6HTVMJ3422AAL/action/author_attestation","sign_citation":"https://pith.science/pith/3BFJ4NWGM6QAJ6HTVMJ3422AAL/action/citation_signature","submit_replication":"https://pith.science/pith/3BFJ4NWGM6QAJ6HTVMJ3422AAL/action/replication_record"}},"created_at":"2026-05-18T00:29:12.087562+00:00","updated_at":"2026-05-18T00:29:12.087562+00:00"}