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arxiv 2112.03312 v4 pith:X2GDKAOB submitted 2021-12-06 cond-mat.str-el

Randomness and Frustration in a S = 1/2 Square-Lattice Heisenberg Antiferromagnet

classification cond-mat.str-el
keywords frustrationmagneticrandomnesscompoundscutegroundheisenbergmeasurements
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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We explore the interplay between randomness and magnetic frustration in the series of $S = 1/2$ Heisenberg square-lattice compounds Sr$_2$CuTe$_{1-x}$W$_x$O$_6$. Substituting W for Te alters the magnetic interactions dramatically, from strongly nearest-neighbor to next-nearest-neighbor antiferromagnetic coupling. We perform neutron scattering measurements to probe the magnetic ground state and excitations over a range of $x$. We propose a bond-disorder model that reproduces ground states with only short-ranged spin correlations in the mixed compounds. The calculated neutron diffraction patterns and powder spectra agree well with the measured data and allow detailed predictions for future measurements. We conclude that quenched randomness plays the major role in defining the physics of Sr$_2$CuTe$_{1-x}$W$_x$O$_6$ with frustration being less significant.

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