Displaced harmonic oscillators with different curvatures produce a predicted extra substructure in vibronic absorption spectra, quantified by a new closed-form Franck-Condon expression; anharmonic and dissipative simulations for H2 and stiff-stilbene illustrate its effects.
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Quantum dissipative systems beyond the standard harmonic model: features of linear absorption and dynamics
Displaced harmonic oscillators with different curvatures produce a predicted extra substructure in vibronic absorption spectra, quantified by a new closed-form Franck-Condon expression; anharmonic and dissipative simulations for H2 and stiff-stilbene illustrate its effects.