RIXS spectra of the Hubbard-SSH model show SSH phonons appearing as multi-particle excitations redshifted below the phonon dispersion, providing a fingerprint for identifying SSH-like interactions.
Theory of electron-phonon interactions in extended correlated systems probed by resonant inelastic x-ray scattering
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abstract
An emerging application of resonant inelastic x-ray scattering (RIXS) is the study of lattice excitations and electron-phonon ($e$-ph) interactions in quantum materials. Despite the growing importance of this area of research, the community lacks a complete understanding of how the RIXS process excites the lattice and how these excitations encode information about the $e$-ph interactions. Here, we present a detailed study of the RIXS spectra of the Hubbard-Holstein model defined on extended one-dimensional lattices. Using the density matrix renormalization group (DMRG) method, we compute the RIXS response while treating the electron mobility, many-body interactions, and core-hole interactions on an equal footing. The predicted spectra exhibit notable differences from those obtained using the commonly adopted Lang-Firsov models, with important implications for analyzing past and future experiments. Our results provide a deeper understanding of how RIXS probes $e$-ph interactions and set the stage for a more realistic analysis of future experiments.
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cond-mat.str-el 1years
2024 1verdicts
CONDITIONAL 1representative citing papers
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Identifying and quantifying Su-Schrieffer-Heeger-like interactions with RIXS
RIXS spectra of the Hubbard-SSH model show SSH phonons appearing as multi-particle excitations redshifted below the phonon dispersion, providing a fingerprint for identifying SSH-like interactions.