C3-symmetric K2IrO3 is predicted to have off-diagonal exchange couplings about ten times larger than Na2IrO3, and exact diagonalization shows such couplings can stabilize spin liquid phases.
Quantum Spin Liquid in a depleted triangular lattice Iridate K$_x$Ir$_y$O$_2$
1 Pith paper cite this work. Polarity classification is still indexing.
abstract
We report discovery of a new iridate family K$_x$Ir$_y$O$_2$ with depleted triangular lattice planes made up of edge sharing IrO$_6$ octahedra separated by K planes. Such a material interpolates between the triangular and honeycomb lattices and is a new playground for Kitaev physics. The materials are Mott insulators with $y = 1 - x/4$. Physical property measurements for the $x \approx 0.85$ material are reported. Using magnetic susceptibility $\chi$ versus temperature $T$ measurements we find $S_{eff} = 1/2$ moments interacting strongly with a Weiss temperature $\theta \approx - 180$~K and no magnetic order or spin freezing down to $T = 1.8$~K\@. Heat capacity shows a broad maximum around $30$~K which is insensitive to magnetic fields and a $T$-linear low temperature behaviour with $\gamma \sim 10$~mJ/mol~K$^2$. These results are consistent with a gapless QSL state in K$_{0.85}$Ir$_{0.79}$O$_2$.
citation-role summary
citation-polarity summary
fields
cond-mat.str-el 1years
2019 1verdicts
CONDITIONAL 1roles
background 1polarities
unclear 1representative citing papers
citing papers explorer
-
Large off diagonal exchange couplings and spin liquid states in $\mathbf{C_3}$ symmetric iridates
C3-symmetric K2IrO3 is predicted to have off-diagonal exchange couplings about ten times larger than Na2IrO3, and exact diagonalization shows such couplings can stabilize spin liquid phases.