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(75) A key point is that all inputs appearing in the equations above —ρ(•),g(2)(•,•),g(3)(•,•,•), g(4)(•,•,•,•)— must be computed under the assumption that the system, environment are decoupled

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physics.chem-ph 1

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2025 1

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CONDITIONAL 1

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A probabilistic approach to system-environment coupling

physics.chem-ph · 2025-04-30 · conditional · novelty 4.0

For pairwise-interacting particles, the mean and variance of the system-environment interaction energy are expressed exactly through up to four-body correlation functions, enabling Gaussian-based free-energy estimates for strongly coupled systems.

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  • A probabilistic approach to system-environment coupling physics.chem-ph · 2025-04-30 · conditional · none · ref 1

    For pairwise-interacting particles, the mean and variance of the system-environment interaction energy are expressed exactly through up to four-body correlation functions, enabling Gaussian-based free-energy estimates for strongly coupled systems.