mPDF analysis reveals persistent ferromagnetic intrachain correlations above TN in CrPS4; when fed into a DFT spin Hamiltonian these correlations drive differential renormalization of single-ion versus exchange anisotropy, rotating the effective easy axis.
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Correlation-Driven Spin Reorientation via Competing Anisotropy Channels in CrPS4
mPDF analysis reveals persistent ferromagnetic intrachain correlations above TN in CrPS4; when fed into a DFT spin Hamiltonian these correlations drive differential renormalization of single-ion versus exchange anisotropy, rotating the effective easy axis.