A bath-engineering quantum simulation framework enables numerically exact 2D spectroscopy calculations for open quantum systems, demonstrated on a driven four-level system and on Rh(CO)2C5H7O2 in chloroform where it reproduces key experimental spectral features.
In addition, the evolution times τ and t vary from 0 to 5 ps, with a time step of 5 fs
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Numerically-Exact Quantum-Simulation Approach for Two-Dimensional Spectroscopy of Open Quantum Systems
A bath-engineering quantum simulation framework enables numerically exact 2D spectroscopy calculations for open quantum systems, demonstrated on a driven four-level system and on Rh(CO)2C5H7O2 in chloroform where it reproduces key experimental spectral features.