Quantum Monte Carlo data on a rubrene-like lattice model show the relaxation time approximation is inconsistent with the computed correlator, while a one-parameter fit yields a low-frequency mobility estimate below RTA and experiment.
Transient localization from the interaction with quantum bosons
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abstract
We carefully revisit the electron-boson scattering problem, going beyond popular semi-classical treatments. By providing numerically exact results valid at finite temperatures, we demonstrate the existence of a regime of electron-boson scattering where quantum localization processes become relevant despite the absence of extrinsic disorder. Localization in the Anderson sense is caused by the emergent randomness resulting from a large thermal boson population, being effective at transient times before diffusion can set in. Compelling evidence of this transient localization phenomenon is provided by the observation of a distinctive displaced Drude peak (DDP) in the optical absorption and the ensuing suppression of conductivity. Our findings identify a general route for anomalous metallic behavior that can broadly apply in interacting quantum matter.
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cond-mat.mtrl-sci 1years
2024 1verdicts
CONDITIONAL 1representative citing papers
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High-precision Quantum Monte-Carlo study of charge transport in a lattice model of molecular organic semiconductors
Quantum Monte Carlo data on a rubrene-like lattice model show the relaxation time approximation is inconsistent with the computed correlator, while a one-parameter fit yields a low-frequency mobility estimate below RTA and experiment.