Water loading flips CO2 adsorption in mmen-Mg2(dobpdc) from cooperative chain growth to isolated-site uptake, and at three waters per diamine a braided H2O/CO2 chain may drive phase-transition-like behavior.
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A combined statistical mechanical and ab initio approach to understanding H2O/CO2 co-adsorption in mmen-Mg2(dobpdc)
Water loading flips CO2 adsorption in mmen-Mg2(dobpdc) from cooperative chain growth to isolated-site uptake, and at three waters per diamine a braided H2O/CO2 chain may drive phase-transition-like behavior.