A broad ab initio grid of CO2–H2/He pressure-broadening data is presented, but the headline 'parameter-free, absolute-scale' validation is achieved only after scaling the theory to experiment.
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Comprehensive Ab Initio Quantum Computations of CO$_{\rm 2}$-H$_{\rm 2}$ and CO$_{\rm 2}$-He Collisional Properties
A broad ab initio grid of CO2–H2/He pressure-broadening data is presented, but the headline 'parameter-free, absolute-scale' validation is achieved only after scaling the theory to experiment.