High-resolution spectroscopy of AlF in the X, a, and A states shows its A1Pi-X1Sigma+ transition is rotationally closed with favorable branching ratios, establishing AlF as a practical laser-cooling candidate.
Magnetically-Trapped Molecules Efficiently Loaded from a Molecular MOT
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abstract
We describe experiments demonstrating efficient transfer of molecules from a magneto-optical trap (MOT) into a conservative magnetic quadrupole trap. Our scheme begins with a blue-detuned optical molasses to cool SrF molecules to $\sim\!50$ $\mu$K. Next, we optically pump the molecules into a strongly-trapped sublevel. This two-step process reliably transfers $64\%$ of the molecules initially trapped in the MOT into the magnetic trap, comparable to similar atomic experiments. Once loaded, the magnetic trap is compressed by increasing the magnetic field gradient. Finally, we demonstrate a magnetic trap lifetime of over $1$ s. This opens a promising new path to the study of ultracold molecular collisions, and potentially the production of quantum-degenerate molecular gases.
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Spectroscopic characterization of aluminum monofluoride with relevance to laser cooling and trapping
High-resolution spectroscopy of AlF in the X, a, and A states shows its A1Pi-X1Sigma+ transition is rotationally closed with favorable branching ratios, establishing AlF as a practical laser-cooling candidate.