A tight-binding dimer model shows that the laser polarization maximizing high-harmonic yield flips from molecular axes to the intermolecular axis at higher orders, with the flip order depending on coupling strength, and this behavior is already present in adiabatically following states.
Also the narrow- ing of the lobes with increasing harmonic order, which was seen in the measurements and theoretical calcula- tions of [25], is reproduced by our dimer model
1 Pith paper cite this work. Polarity classification is still indexing.
1
Pith paper citing it
fields
quant-ph 1years
2025 1verdicts
UNVERDICTED 1representative citing papers
citing papers explorer
-
High-harmonic generation from two weakly coupled molecules: a simple tight-binding model
A tight-binding dimer model shows that the laser polarization maximizing high-harmonic yield flips from molecular axes to the intermolecular axis at higher orders, with the flip order depending on coupling strength, and this behavior is already present in adiabatically following states.