Spin-group symmetry analysis and first-principles calculations excluding SOC on monolayer 2H-VS2 demonstrate that collinear stripy antiferromagnetic order induces 25 μC/cm² in-plane ferroelectric polarization via SOC-independent p-d hybridization.
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Colossal Type-II Multiferroic Polarization Driven by Collinear Spin Orders
Spin-group symmetry analysis and first-principles calculations excluding SOC on monolayer 2H-VS2 demonstrate that collinear stripy antiferromagnetic order induces 25 μC/cm² in-plane ferroelectric polarization via SOC-independent p-d hybridization.