Multilayered materials extend exciton-polariton coherence lifetime and enhance transport versus single layers at fixed Rabi splitting via phonon fluctuation synchronization that suppresses dynamical disorder.
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A mean-field pump-probe model shows that dephasing-generated dark exciton populations slow the measured root-mean-square transport of molecular cavity polaritons below their group velocity.
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Exciton-Polariton Dynamics in Multilayered Materials
Multilayered materials extend exciton-polariton coherence lifetime and enhance transport versus single layers at fixed Rabi splitting via phonon fluctuation synchronization that suppresses dynamical disorder.
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Mapping molecular polariton transport via pump-probe microscopy
A mean-field pump-probe model shows that dephasing-generated dark exciton populations slow the measured root-mean-square transport of molecular cavity polaritons below their group velocity.