Collective vibrational strong coupling in a simulated (H2O)21-cavity system delocalizes OH stretches and opens new intermolecular energy pathways, with efficiency set by transition-dipole alignment with the cavity field.
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Quantum mechanical deconstruction of vibrational energy transfer rate and pathways modified by collective vibrational strong coupling
Collective vibrational strong coupling in a simulated (H2O)21-cavity system delocalizes OH stretches and opens new intermolecular energy pathways, with efficiency set by transition-dipole alignment with the cavity field.