The coupling to center-of-mass motion shifts and weakens the avoided crossings used for mergoassociation and requires a new shifted-molecule basis set for efficient calculations.
7 is the motional coupling be- tween relative and center-of-mass motions, characterized by ∆ω2
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Making molecules by mergoassociation: the role of center-of-mass motion
The coupling to center-of-mass motion shifts and weakens the avoided crossings used for mergoassociation and requires a new shifted-molecule basis set for efficient calculations.