Resonant THz excitation of Ce3+ crystal-field levels in paramagnetic CeF3 produces long-lived helicity-odd magnetization whose spectral sign reversal matches resonant inverse-Faraday theory.
The crystal was double-side polished with a (001) crystal orientation, such that the crystallographic c- axis (optical axis) was normal to the surface
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A crystal-field route to THz-driven magnetization
Resonant THz excitation of Ce3+ crystal-field levels in paramagnetic CeF3 produces long-lived helicity-odd magnetization whose spectral sign reversal matches resonant inverse-Faraday theory.