Molecular aggregates coupled to polaritons show superradiance enhanced beyond Dicke's N scaling, with a general analytical rate expression derived for dispersive and absorbing media.
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Simulations show non-resonant pump-probe schemes retain high sensitivity to strongly-coupled molecules while being less prone to optical artifacts than resonant schemes.
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Anomalous Giant Superradiance in Molecular Aggregates Coupled to Polaritons
Molecular aggregates coupled to polaritons show superradiance enhanced beyond Dicke's N scaling, with a general analytical rate expression derived for dispersive and absorbing media.
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Nonlinear signal enhancement of strongly-coupled molecules in pump-probe experiments
Simulations show non-resonant pump-probe schemes retain high sensitivity to strongly-coupled molecules while being less prone to optical artifacts than resonant schemes.