For non-Markovian dynamics, the maximal transition-path probability is non-monotonic in memory time and can exceed 1/2, invalidating 1/2 as a universal reaction-coordinate quality benchmark.
Peters, Reaction Coordinates and Mechanistic Hypoth- esis Tests, Annu
1 Pith paper cite this work. Polarity classification is still indexing.
1
Pith paper citing it
citation-role summary
background 1
citation-polarity summary
fields
physics.chem-ph 1years
2025 1verdicts
CONDITIONAL 1roles
background 1polarities
unclear 1representative citing papers
citing papers explorer
-
Non-Markovianity increases transition path probability
For non-Markovian dynamics, the maximal transition-path probability is non-monotonic in memory time and can exceed 1/2, invalidating 1/2 as a universal reaction-coordinate quality benchmark.