Realistic exciton-phonon coupling is too weak for Dyakonov-Perel motional narrowing in MoS2; full-Brillouin-zone intervalley scattering shortens valley depolarization 3–4× to ~50 fs (300 K) and ~130 fs (10 K).
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2 Pith papers cite this work, alongside 49 external citations. Polarity classification is still indexing.
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This perspective article develops a definition of foundational MLIPs and poses six open questions that the authors believe will define future research in machine-learned interatomic potentials.
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Exciton valley depolarization in monolayer MoS2: non-Markovian quantum dynamics, intervalley scattering, and the breakdown of the Dyakonov-Perel mechanism
Realistic exciton-phonon coupling is too weak for Dyakonov-Perel motional narrowing in MoS2; full-Brillouin-zone intervalley scattering shortens valley depolarization 3–4× to ~50 fs (300 K) and ~130 fs (10 K).
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Six Open Questions in Machine-Learned Interatomic Potential Foundation Models
This perspective article develops a definition of foundational MLIPs and poses six open questions that the authors believe will define future research in machine-learned interatomic potentials.