Vibrational strong coupling produces resonant changes to vibrationally-resolved London dispersion forces that enhance reaction rates for two molecules coupled to a cavity mode.
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physics.chem-ph 2years
2026 2verdicts
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In the Tavis-Cummings model, collective dynamics are linear at vanishing excitation density and nonlinear at finite density, with mean-field accurate for large N while cluster expansion captures finite-N effects.
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Resonant and collective modification of London dispersion interactions under vibrational strong coupling
Vibrational strong coupling produces resonant changes to vibrationally-resolved London dispersion forces that enhance reaction rates for two molecules coupled to a cavity mode.
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Excitation density controlled regimes of collective light--matter dynamics
In the Tavis-Cummings model, collective dynamics are linear at vanishing excitation density and nonlinear at finite density, with mean-field accurate for large N while cluster expansion captures finite-N effects.