Spacers in aza-BODIPY dimers reduce excessive state mixing, promote distinct multiexcitonic states, and tune singlet fission rates over several orders of magnitude via substitution and conjugation patterns.
Mild Open-shell Character of BODIPY and Its Impact on Singlet and Triplet Excitation Energies.J
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Design Principles for Singlet Fission in Aza-BODIPY Dimers: Spacer-Controlled Electronic Structure and Energy Ordering
Spacers in aza-BODIPY dimers reduce excessive state mixing, promote distinct multiexcitonic states, and tune singlet fission rates over several orders of magnitude via substitution and conjugation patterns.