The change of a diffusion activation barrier with temperature equals the variance of site energies, minus the variance of transition-state energies, plus a kinetic correlation term (Eq. 5).
High-entropy strategy flattening lithium ion migration energy landscape to enhance the conductivity of garnet-type solid-state electrolytes,
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Statistical Mechanics of Thermal Diffusion in Rough Energy Landscapes
The change of a diffusion activation barrier with temperature equals the variance of site energies, minus the variance of transition-state energies, plus a kinetic correlation term (Eq. 5).