Shake-down satellites in time-resolved XPS of CS2 are spin-selective for singlet states, enabling assignment of the 1B2[1Δu] intermediate and its ~350 fs internal conversion.
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Shake-down spectroscopy as state- and site-specific probe of ultrafast chemical dynamics
Shake-down satellites in time-resolved XPS of CS2 are spin-selective for singlet states, enabling assignment of the 1B2[1Δu] intermediate and its ~350 fs internal conversion.