USb2 is characterized as the first high-temperature singlet ground state magnet enabled by Hund's rule correlations, with experimental signatures from X-ray dichroism and neutron scattering interpreted via theoretical analysis as resembling exciton condensation.
et al., WIEN2k edited by Technische Universität Wien Austria, 2001 Acknowledgements: We are grateful for discussions with S
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High temperature singlet-based magnetism from Hund's rule correlations
USb2 is characterized as the first high-temperature singlet ground state magnet enabled by Hund's rule correlations, with experimental signatures from X-ray dichroism and neutron scattering interpreted via theoretical analysis as resembling exciton condensation.