Tailored cubic spectral phase on femtosecond pulses compresses rotational revivals to enable direct time-domain observation of l-doubling contributions previously obscured by centrifugal distortion.
Kierspel et al., X-Ray Diffractive Imaging of Controlled Gas-Phase Molecules: Toward Imaging of Dynamics in the Molecular Frame, J
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Direct Time-Domain Observation of l-Doubling via Centrifugal-Distortion Pre-compensation
Tailored cubic spectral phase on femtosecond pulses compresses rotational revivals to enable direct time-domain observation of l-doubling contributions previously obscured by centrifugal distortion.