Sn incorporation in MBA₂SnₓPb₁₋ₓI₄ distorts octahedra with only minor effect on structural chirality while substantially enhancing phonon chirality, yet without increasing temperature-gradient angular momentum due to mode compensation.
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Molecular dynamics with ML force fields shows inorganic layers in MBA2PbI4 lose chirality faster than organic cations with rising temperature due to hydrogen bond breaking.
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Impact of Metal Cation on Chiral Properties of 2D Halide Perovskites
Sn incorporation in MBA₂SnₓPb₁₋ₓI₄ distorts octahedra with only minor effect on structural chirality while substantially enhancing phonon chirality, yet without increasing temperature-gradient angular momentum due to mode compensation.
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Temperature-Dependent Chirality in Halide Perovskites
Molecular dynamics with ML force fields shows inorganic layers in MBA2PbI4 lose chirality faster than organic cations with rising temperature due to hydrogen bond breaking.