A tunable microscopic model of network liquids with a liquid-liquid phase transition, analyzed via RFOT theory, predicts nanonucleation near the glass transition and links thermodynamic and kinetic anomalies when matched to water-like conditions.
and Kearns, Kenneth L
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cond-mat.soft 2years
2026 2verdicts
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Vapor deposition experiments show 2-ethyl-1-hexanol glass kinetic stability rises sharply with slower deposition rates, attributed to surface mobility more than 4 orders of magnitude lower than ethylcyclohexane at 0.85 Tg.
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Polyamorphism in Glassy Network Materials
A tunable microscopic model of network liquids with a liquid-liquid phase transition, analyzed via RFOT theory, predicts nanonucleation near the glass transition and links thermodynamic and kinetic anomalies when matched to water-like conditions.
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Limited surface mobility inhibits stable glass formation for 2-ethyl-1-hexanol
Vapor deposition experiments show 2-ethyl-1-hexanol glass kinetic stability rises sharply with slower deposition rates, attributed to surface mobility more than 4 orders of magnitude lower than ethylcyclohexane at 0.85 Tg.