The authors derive mean-field and mapping-variable ring polymer instantons for multistate systems and show that mean-field rates match Fermi's Golden Rule and adiabatic instanton benchmarks across coupling regimes.
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Multistate ring polymer instantons and nonadiabatic reaction rates
The authors derive mean-field and mapping-variable ring polymer instantons for multistate systems and show that mean-field rates match Fermi's Golden Rule and adiabatic instanton benchmarks across coupling regimes.