Ligand holes on planar and apical oxygen hybridize selectively with Ni d_x2-y2 and d_z2 orbitals in La4Ni3O10, enabling RIXS to show d_x2-y2 dominance in low-energy excitations and a ~50 meV interlayer superexchange from observed bimagnons.
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Distinct orbital contributions to electronic and magnetic structures in La$_{4}$Ni$_{3}$O$_{10}$
Ligand holes on planar and apical oxygen hybridize selectively with Ni d_x2-y2 and d_z2 orbitals in La4Ni3O10, enabling RIXS to show d_x2-y2 dominance in low-energy excitations and a ~50 meV interlayer superexchange from observed bimagnons.