Opposite sub-cycle correlation dynamics appear in noble-gas versus alkaline-earth atoms, and the correlation-driven evolution of natural orbitals, rather than occupation numbers, dominates the HHG spectrum.
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Reduced density matrix description of high-harmonic generation in multi-electron atoms: exploring sub-cycle correlation effects
Opposite sub-cycle correlation dynamics appear in noble-gas versus alkaline-earth atoms, and the correlation-driven evolution of natural orbitals, rather than occupation numbers, dominates the HHG spectrum.