Attosecond transient absorption on Cu-poor CIGS reveals coherent A1g phonons in chalcopyrite and ordered vacancy compound phases, and 18.6 fs oscillations attributed to electronic quantum path interference between their conduction bands.
Long-Lived Coherence between Incoherent Excitons revealed by Time-Resolved ARPES: An Exact Solution
1 Pith paper cite this work. Polarity classification is still indexing.
abstract
We investigate the exciton dynamics in an exactly solvable two-band model for semiconductors. The model incorporates light-matter, electron-electron and electron-phonon interactions, and captures exciton formation as well as the transition from the coherent to the incoherent regime. We analyze excitonic polarization, populations and coherences, with special focus on their impact in Time-Resolved and Angle-Resolved Photoemission Spectroscopy (TR-ARPES). For nonresonant pumping with below-gap photon energies, TR-ARPES spectra reveal distinct excitonic replica and quantum beats persisting in the incoherent regime. These are due to a coherence between different species of {\em incoherent} excitons. Such type of coherence is resistant to phonon dephasing, indicating that it follows different dynamics than those governing the coherences considered so far.
citation-role summary
citation-polarity summary
fields
cond-mat.mtrl-sci 1years
2025 1verdicts
CONDITIONAL 1roles
background 1polarities
unclear 1representative citing papers
citing papers explorer
-
Coherent phonon motions and ordered vacancy compound mediated quantum path interference in Cu-poor CuIn$_{x}$Ga$_{(1-x)}$Se$_2$ (CIGS) with attosecond transient absorption
Attosecond transient absorption on Cu-poor CIGS reveals coherent A1g phonons in chalcopyrite and ordered vacancy compound phases, and 18.6 fs oscillations attributed to electronic quantum path interference between their conduction bands.