Pulsed driving of molecular polaritons produces vibrational excitation with linear (quadratic in field amplitude) and nonlinear (quartic in field amplitude) contributions whose microscopic origin is an intrapulse polariton-mediated stimulated Raman process.
In practice, we choosetp = 100 fs for the ultrashort- pulse excitation andt p = 1000 fs for the long-pulse excitation
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Linear and nonlinear vibrational excitation driven by molecular polaritons
Pulsed driving of molecular polaritons produces vibrational excitation with linear (quadratic in field amplitude) and nonlinear (quartic in field amplitude) contributions whose microscopic origin is an intrapulse polariton-mediated stimulated Raman process.