Polarization-controlled spectroscopy on conformationally flexible pentacene dimers shows persistent singlet-triplet mixing in the bound (TT1)1 state across bridging motifs, with decorrelation outcompeted by decay.
D.et al.Exciton delocalization drives rapid singlet fission in nanopar- ticles of acene derivatives.Journal of the American Chemical Society137, 45 6790–6803 (2015)
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Persistent singlet electronic character in the multiexcitonic triplet-pair state of strongly coupled pentacene singlet fission dimers
Polarization-controlled spectroscopy on conformationally flexible pentacene dimers shows persistent singlet-triplet mixing in the bound (TT1)1 state across bridging motifs, with decorrelation outcompeted by decay.