The paper derives exact thermodynamic relations for strongly coupled open systems under a zero-variance interaction condition, expressing free energy and internal energy through the interaction-energy distribution and a chi-squared divergence.
( 9), we obtain after simplification ZS+E Z ∗ ZE = ⟨exp(−2βV SE )⟩E0 ⟨exp(−βV SE )⟩2 E|S
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Thermodynamic potentials from a probabilistic view on the system-environment interaction energy
The paper derives exact thermodynamic relations for strongly coupled open systems under a zero-variance interaction condition, expressing free energy and internal energy through the interaction-energy distribution and a chi-squared divergence.