A thermodynamic model of hydration and ion association in the EDL of WiSEs rationalizes expanded electrochemical stability windows via Nernst bulk activity and Butler-Volmer interface kinetics effects.
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A theory of Li+ solvation in the Helmholtz layer, parameterized from bulk MD, finds binding probabilities remain equal to bulk values, supporting bulk solvation as a proxy for SEI studies.
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Thermodynamic effects of solid electrolyte interphase formation from solvation and ionic association in water-in-salt electrolytes
A thermodynamic model of hydration and ion association in the EDL of WiSEs rationalizes expanded electrochemical stability windows via Nernst bulk activity and Butler-Volmer interface kinetics effects.
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Theory of Cation Solvation in the Helmholtz Layer of Li-ion Battery Electrolytes
A theory of Li+ solvation in the Helmholtz layer, parameterized from bulk MD, finds binding probabilities remain equal to bulk values, supporting bulk solvation as a proxy for SEI studies.