The superconducting dome in electron-doped MoS2 is recreated from first principles and traced to the 1x1 H to 2x2 charge-density-wave transition and later structural phases.
Long living carriers in a strong electron-phonon interacting two-dimensional doped semiconductor
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abstract
Carrier doping by the electric field effect has emerged recently as an ideal route for monitoring many-body physics in two-dimensional (2D) materials where the Fermi level is tuned in a way that -- indirectly -- the strength of the interactions can also be scanned. The possibility of systematic doping in combination with high resolution photoemission has allowed to uncover a genuinely many-body electron spectrum in single-layer MoS2 transition metal dichalcogenide, resolving three clear quasi-particle states, where only one state should be expected if the electron-phonon interaction vanished. Our analysis combines first-principles and consistent complex plane analytic approaches and brings into light the presence and the physical origin of two gaps and the three quasi-particle bands which are unambiguously present in the photoemission spectrum. One of these states, though being strongly interacting with the accompanying virtual phonon cloud, presents a notably long lifetime which is an appealing property when trying to understand and take advantage of many-body interactions to modulate the transport properties.
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Understanding the origin of superconducting dome in electron-doped MoS$_2$ monolayer
The superconducting dome in electron-doped MoS2 is recreated from first principles and traced to the 1x1 H to 2x2 charge-density-wave transition and later structural phases.