In slow spectral diffusion, photon intensity and fluctuations depend on nonequilibrium environmental traits at short times but become independent in steady state; in fast diffusion, line shape and Mandel's parameter are independent of nonequilibrium characteristics due to rapid relaxation.
In this case, the photon emission of the driven single molecule cannot respond instantaneously to the relaxation of nonequilibrium environmental fluctuations
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Photon counting statistics in the presence of spectral diffusion induced by nonequilibrium environmental fluctuations
In slow spectral diffusion, photon intensity and fluctuations depend on nonequilibrium environmental traits at short times but become independent in steady state; in fast diffusion, line shape and Mandel's parameter are independent of nonequilibrium characteristics due to rapid relaxation.