Pulsed driving of molecular polaritons produces vibrational excitation with linear (quadratic in field amplitude) and nonlinear (quartic in field amplitude) contributions whose microscopic origin is an intrapulse polariton-mediated stimulated Raman process.
One observes that the resonance of the ground-state vibrational responseP g,ν=1 is extremely sharp (due to the nature of resonant driven oscillator), as shown in Fig
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Linear and nonlinear vibrational excitation driven by molecular polaritons
Pulsed driving of molecular polaritons produces vibrational excitation with linear (quadratic in field amplitude) and nonlinear (quartic in field amplitude) contributions whose microscopic origin is an intrapulse polariton-mediated stimulated Raman process.