Stochastic density functional theory on Brownian particles yields a generalized Langevin equation for ionic charge density with solvent-mediated memory, producing simple dynamical structure factors under timescale separation and predicting two-step relaxation for slow solvents.
Within our description and approxi- mations, thetransverserelaxation time is simply given by 1/(DSq2 + 2Dr S) [46, 55]
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Solvent-induced memory effects in a model electrolyte
Stochastic density functional theory on Brownian particles yields a generalized Langevin equation for ionic charge density with solvent-mediated memory, producing simple dynamical structure factors under timescale separation and predicting two-step relaxation for slow solvents.