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arxiv: 1210.8187 · v1 · submitted 2012-10-30 · ❄️ cond-mat.str-el

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Quantum Tunneling in Half-Integer-Spin Kagome-Lattice Langasites

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classification ❄️ cond-mat.str-el
keywords half-integer-spinkagome-latticemagneticmuonquantumrelaxationspintunneling
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Employing the muon spin relaxation technique we evidence temperature independent magnetic fluctuations persisting down to the lowest temperatures in the samarium-based ($J=5/2$) kagome-lattice Langasite. A detailed bulk-magnetization characterization and comparison to the neodymium-based ($J=9/2$) compound allow us to assign the persistent spin dynamics to a quantum tunneling process. This is facilitated by pairwise anisotropic magnetic interactions, leading to a universal scaling of the muon relaxation. Our study reveals a remarkable analogy between weakly interacting half-integer-spin rare-earth magnets and molecular nanomagnets.

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