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arxiv: 1211.3236 · v1 · pith:6NBKKFK6new · submitted 2012-11-14 · ❄️ cond-mat.str-el

Ultrafast charge recombination in photoexcited Mott-Hubbard insulator

classification ❄️ cond-mat.str-el
keywords mott-hubbardrecombinationbackboundcalculationchargeconsequentlycorrelations
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We present a calculation of the recombination rate of the excited holon-doublon pairs based on the two-dimensional model relevant for undoped cuprates which shows that fast processes, observed in pump-probe experiments on Mott-Hubbard insulators in picosecond range, can be explained even quantitatively with the multi-magnon emission. The precondition is the existence of the Mott-Hubbard bound exciton of the s-type. We find that its decay is exponentially dependent on the Mott-Hubbard gap and on the magnon energy, with a small prefactor which can be traced back to strong correlations and consequently large exciton-magnon coupling.

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