Doppler-free intermodulated fluorescence spectroscopy of ⁴He 2³P-3^(1,3)D transitions at 588 nm with a one-watt compact laser system
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We have demonstrated Doppler-free intermodulated fluorescence spectroscopy of helium $2^3P-3^{1,3}D$ transitions in an rf discharged sealed-off cell using a compact laser system at 588 nm. An external cavity diode laser at 1176 nm was constructed to seed a Raman fiber amplifier. Laser power of more than one watt at 588 nm was produced by frequency doubling of the fiber amplifier output using a MgO:PPLN crystal. A doubling efficiency of 23 % was achieved. The power-dependent spectra of the $2^3P-3^3D$ transitions were investigated. Furthermore, the Doppler-free spectrum of the spin-forbidden $2^3P-3^1D$ transitions was observed for the first time. Our results are crucial towards precision test of QED atomic calculations, especially for improving the determination of the helium $3^1D-3^3D$ separation.
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