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arxiv: 1610.05337 · v1 · pith:SFEBSZCXnew · submitted 2016-10-17 · ❄️ cond-mat.str-el

Observation of semi-localized dispersive states in the strongly correlated electron-doped ferromagnet Eu_(1-x)Gd_(x)O

classification ❄️ cond-mat.str-el
keywords dopedcomplexcuriedopingsemi-localizedstatesstudiestemperature
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Chemical substitution plays a key role in controlling the electronic and magnetic properties of complex materials. For instance, in EuO, carrier doping can induce a spin-polarized metallic state, colossal magnetoresistance, and significantly enhance the Curie temperature. Here, we employ a combination of molecular-beam epitaxy, angle-resolved photoemission spectroscopy, and an effective model calculation to investigate and understand how semi-localized states evolve in lightly electron doped Eu$_{1-x}$Gd$_{x}$O above the ferromagnetic Curie temperature. Our studies reveal a characteristic length scale for the spatial extent of the donor wavefunctions which remains constant as a function of doping, consistent with recent tunneling studies of doped EuO. Our work sheds light on the nature of the semiconductor-to-metal transition in Eu$_{1-x}$Gd$_{x}$O and should be generally applicable for doped complex oxides.

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