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arxiv: 1706.03326 · v1 · pith:GI6DDPMUnew · submitted 2017-06-11 · ❄️ cond-mat.str-el

Transitions from a Kondo-like diamagnetic insulator into a modulated ferromagnetic metal in bm{FeGa_{3-y}Ge_y}

classification ❄️ cond-mat.str-el
keywords ferromagneticfegaitinerantmagneticmetalweaklydiamagneticlocalized
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One initial and essential question of magnetism is whether the magnetic properties of a material are governed by localized moments or itinerant electrons. Here we expose the case for the weakly ferromagnetic system FeGa$_{3-y}$Ge$_y$ wherein these two opposite models are reconciled, such that the magnetic susceptibility is quantitatively explained by taking into account the effects of spin-spin correlation. With the electron doping introduced by Ge substitution, the diamagnetic insulating parent compound FeGa$_3$ becomes a paramagnetic metal as early as at $ y=0.01 $, and turns into a weakly ferromagnetic metal around the quantum critical point $ y=0.15 $. Within the ferromagnetic regime of FeGa$_{3-y}$Ge$_y$, the magnetic properties are of a weakly itinerant ferromagnetic nature, located in the intermediate regime between the localized and the itinerant dominance. Our analysis implies a potential universality for all itinerant-electron ferromagnets.

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